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"Heusler compounds, with a general composition X2YZ (with X, Y being a transition metal and Z an element from the III-V groups) are attracting an interest due to their possible use in the novel field of spin-dependent devices, also known as spintronics. This interest in Heusler compounds comes from the half-metallic character of their spin-split band structure, i.e. metallic behavior for one spin ...